Ultrafast Science, Volume. 4, Issue 1, 0064(2024)

Efficient Optical Control of Magnon Dynamics in van der Waals Ferromagnets

Yu Gong1、*, Zhonghua Yang2,3, Alem Teklu1, Ti Xie4, Noah Kern1, Andrew F. May5, Michael McGuire5, Christian Brennan1, Er-Jia Guo6, Narayanan Kuthirummal1, John Cetin1, Qian Zhang1, Ming Hu2, and Cheng Gong4
Author Affiliations
  • 1Department of Physics and Astronomy, College of Charleston, Charleston, SC 29424, USA.
  • 2Department of Mechanical Engineering, University of South Carolina, Columbia, SC 29208, USA.
  • 3College of Architecture and Civil Engineering, Shenyang University of Technology, Shenyang 110870, China.
  • 4Department of Electrical and Computer Engineering and Quantum Technology Center, University of Maryland, College Park, MD 20742, USA.
  • 5Materials Science and Technology Division, Oak Ridge National Laboratory, Oak Ridge, TN 37831, USA.
  • 6Beijing National Laboratory for Condensed Matter Physics and Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China.
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    Optical control of magnons in two-dimensional (2D) materials promises new functionalities for spintronics and magnonics in atomically thin devices. Here, we report control of magnon dynamics, using laser polarization, in a ferromagnetic van der Waals (vdW) material, Fe3.6Co1.4GeTe2. The magnon amplitude, frequency, and lifetime are controlled and monitored by time-resolved pump-probe spectroscopy. We show substantial (over 25%) and continuous modulation of magnon dynamics as a function of incident laser polarization. Our results suggest that the modification of the effective demagnetization field and magnetic anisotropy by the pump laser pulses with different polarizations is due to anisotropic optical absorption. This implies that pump laser pulses modify the local spin environment, which enables the launch of magnons with tunable dynamics. Our first-principles calculations confirm the anisotropic optical absorption of different crystal orientations. Our findings suggest a new route for the development of opto-spintronic or opto-magnonic devices.

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    Yu Gong, Zhonghua Yang, Alem Teklu, Ti Xie, Noah Kern, Andrew F. May, Michael McGuire, Christian Brennan, Er-Jia Guo, Narayanan Kuthirummal, John Cetin, Qian Zhang, Ming Hu, Cheng Gong. Efficient Optical Control of Magnon Dynamics in van der Waals Ferromagnets[J]. Ultrafast Science, 2024, 4(1): 0064

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    Paper Information

    Category: Research Articles

    Received: Oct. 24, 2023

    Accepted: May. 8, 2024

    Published Online: Dec. 13, 2024

    The Author Email: Gong Yu (gongy@cofc.edu)

    DOI:10.34133/ultrafastscience.0064

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