Acta Optica Sinica, Volume. 32, Issue 6, 619006(2012)

Ultraviolet-Light-Induced Absorption and Its Relaxation in Fe-Doped Near-Stoichiometric LiNbO3

Zhang Yanli*, Liu Youwen, Yang Yongmei, and He Chongjun
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  • [in Chinese]
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    Near-stoichiometric lithium niobate (SLN) crystals doped with low iron are grown, in which the mass fractions of iron are 0×10-6, 5×10-6, 10×10-6, 25×10-6, 50×10-6, 100×10-6, respectively. And their ultraviolet-visible transmission spectra are measured. The concentrations of Fe2+ and Fe3+ are estimated by the linear absorption coefficients at the wavelength of 477 nm. The dynamic process and steady characteristics of the light-induced absorption of crystals are investigated by the pump-probe (365 nm and 632.8 nm) method. The results show that the dark decay process of light-induced absorption exhibits a stretched-exponential behavior, and the decay time constant (i.e., the small polaron lifetime) decreases with the Fe-doped concentration and the pump intensity, while the stretching factor decreases with the pumping intensity. The electron transport equations are solved numerically by the four-order Runge-Kutta method, and the whole process of the light-induced absorption in the SLN crystals doped with Fe is simulated, which is consistent with the experimental results.

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    Zhang Yanli, Liu Youwen, Yang Yongmei, He Chongjun. Ultraviolet-Light-Induced Absorption and Its Relaxation in Fe-Doped Near-Stoichiometric LiNbO3[J]. Acta Optica Sinica, 2012, 32(6): 619006

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    Paper Information

    Category: Nonlinear Optics

    Received: Feb. 20, 2012

    Accepted: --

    Published Online: May. 2, 2012

    The Author Email: Yanli Zhang (zhangyanli0117@126.com)

    DOI:10.3788/aos201232.0619006

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