Ultrafast Science, Volume. 4, Issue 1, 0073(2024)
Probing Coupled Rotational and Electronic Dynamics during Laser-Induced Molecular Fragmentation
Coupled nuclear and electronic dynamics within a molecule are key to understanding a broad range of fundamental physical and chemical processes. Although probing the coupled vibrational and electronic dynamics was demonstrated, it has so far been challenging to observe the coupling interactions between the rotational and electronic degrees of freedom. Here, we report the first observation of Coriolis coupling, a coupling interaction between nuclear rotational angular momentum and electronic axial angular momentum, during laser-induced molecular fragmentation by tracing the electronic structure of a dissociating
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Keyu Guo, Xiaoqing Hu, Min Li, Cong-Cong Jia, Songbin Zhang, Chuanpeng Cao, Wenhai Xie, Wei Cao, Kunlong Liu, Yueming Zhou, Yong Wu, Jianguo Wang, Peixiang Lu. Probing Coupled Rotational and Electronic Dynamics during Laser-Induced Molecular Fragmentation[J]. Ultrafast Science, 2024, 4(1): 0073
Category: Research Articles
Received: Mar. 27, 2024
Accepted: Jul. 26, 2024
Published Online: Dec. 13, 2024
The Author Email: Li Min (mli@hust.edu.cn), Wu Yong (wu_yong@iapcm.ac.cn), Lu Peixiang (lupeixiang@hust.edu.cn)