The prediction of color appearance is the basic theory and technology in modern color science field. To evaluate the color appearance of low-glossiness color printing atlas Liyin offset paper color printing atlas is taken as the experimental samples. Then based on color science and visual psychophysics methods, datasets of the samples′ color appearance are established. The mathematical statistics methods, correlation coefficient R2 and coefficient of variation CV, are used to evaluate the visual prediction results of Y-M in this color atlas under three different light sources. The experiment shows that the results are very different between A and the other two kinds of light sources, D65 and TL84. All findings indicate that the assessment of lightness and hue is more accurate than chroma.