Acta Photonica Sinica, Volume. 51, Issue 8, 0851511(2022)
Ultrafast Two-dimensional Electronic Spectroscopy and Excited-state Dynamics(Invited)
Ultrafast Two-Dimensional Electronic Spectroscopy (2DES) has emerged as a powerful tool to probe excited-state dynamics in photosynthesis, photovoltaic materials, quantum dots, and two-dimensional materials in recent years. Compared to one-dimensional time-resolved spectroscopy, 2DES not only contains one additional dimension to resolve excited-state dynamics but also provides rich information about homogeneous and inhomogeneous broadening, intermolecular coupling and coherent dynamics that are not fully accessible to the traditional third-order spectroscopic methods. Here we will briefly introduce the principle of 2DES from the basic concepts such as Fourier-transform linear spectroscopy, and transient grating. Subsequently, we will illustrate the applications of 2DES in the context of recent studies of spectral broadening in two-dimensional materials, and charge separation and coherent dynamics in photosynthesis and photovoltaic materials. Finally, we will discuss the remaining challenges and exciting future directions for the fields of 2DES.
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Yin SONG, Ruidan ZHU, Shuang YU, Xiaojuan CHUAI, Lirong QIU, Weiqian ZHAO. Ultrafast Two-dimensional Electronic Spectroscopy and Excited-state Dynamics(Invited)[J]. Acta Photonica Sinica, 2022, 51(8): 0851511
Category: Special Issue for the 60th Anniversary of XIOPM of CAS, and the 50th Anniversary of the Acta Photonica Sinica Ⅱ
Received: Jul. 25, 2022
Accepted: Aug. 11, 2022
Published Online: Oct. 25, 2022
The Author Email: ZHAO Weiqian (zwq669@126.com)